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dc.date.accessioned | 2021-10-13T17:41:06Z | |
dc.date.available | 2021-10-13T17:41:06Z | |
dc.date.issued | 2005-01 | |
dc.identifier.uri | http://sedici.unlp.edu.ar/handle/10915/126591 | |
dc.description.abstract | We report on a Ni L2,3 edge x-ray absorption spectroscopy study in RNiO₃ perovskites. These compounds exhibit a metal-to-insulator (MI) transition as temperature decreases. The L₃ edge presents a clear splitting in the insulating state, associated to a less hybridized ground state. Using charge transfer multiplet calculations, we establish the importance of the crystal field and 3d spin-orbit coupling to create a mixed-spin ground state. We explain the MI transition in RNiO₃ perovskites in terms of modifications in the Ni³⁺ crystal field splitting that induces a spin transition from an essentially low-spin to a mixed-spin state. | en |
dc.language | en | es |
dc.subject | spectroscopy | es |
dc.subject | x-ray absorption | es |
dc.subject | crystal field | es |
dc.subject | 3d spin-orbit coupling | es |
dc.subject | perovskites | es |
dc.title | Spin-orbit-induced mixed-spin ground state in RNiO₃ perovskites probed by x-ray absorption spectroscopy: Insight into the metal-to-insulator transition | en |
dc.type | Articulo | es |
sedici.identifier.other | arXiv:cond-mat/0412276 | es |
sedici.identifier.other | doi:10.1103/physrevb.71.020406 | es |
sedici.identifier.issn | 1098-0121 | es |
sedici.identifier.issn | 1550-235X | es |
sedici.creator.person | Piamonteze, Cinthia | es |
sedici.creator.person | Groot, F. M. F. de | es |
sedici.creator.person | Tolentino, Hélio C. N. | es |
sedici.creator.person | Ramos, A. Y. | es |
sedici.creator.person | Massa, Néstor Emilio | es |
sedici.creator.person | Alonso, José Antonio | es |
sedici.creator.person | Martínez Lope, María Jesús | es |
sedici.subject.materias | Ciencias Exactas | es |
sedici.subject.materias | Física | es |
sedici.subject.materias | Química | es |
sedici.description.fulltext | true | es |
mods.originInfo.place | Facultad de Ciencias Exactas | es |
mods.originInfo.place | Centro de Química Inorgánica | es |
sedici.subtype | Articulo | es |
sedici.rights.license | Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0) | |
sedici.rights.uri | http://creativecommons.org/licenses/by-nc-sa/4.0/ | |
sedici.description.peerReview | peer-review | es |
sedici.workflowEdited | true | es |
sedici.relation.journalTitle | Physical Review B | es |
sedici.relation.journalVolumeAndIssue | vol. 71, no. 2 | es |